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New insight into effect of potential on degradation of Fe-N-C catalyst for ORR

Yanyan GAO, Manman QI, Liang HE, Haiping CHEN, Wenzhe LUO, Ming HOU, Zhigang SHAO

Frontiers in Energy 2021, Volume 15, Issue 2,   Pages 421-430 doi: 10.1007/s11708-021-0727-2

Abstract: In recent years, Fe-N-C catalyst is particularly attractive due to its high oxygen reduction reactionHowever, the durability problems still pose challenge to the application of Fe-N-C catalyst.Although considerable work has been done to investigate the degradation mechanisms of Fe-N-C catalystIn fact, the 2e pathway in the ORR process of Fe-N-C catalyst would result in the formation of H O ,In this paper, a new insight into the effect of potential on degradation of Fe-N-C catalyst was provided

Keywords： proton exchange membrane fuel cells (PEMFCs)     oxygen reduction reaction (ORR)     Fe-N-C catalyst     potential    

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Influence of Fe on electrocatalytic activity of iron-nitrogen-doped carbon materials toward oxygen reduction

Lin LI, Cehuang FU, Shuiyun SHEN, Fangling JIANG, Guanghua WEI, Junliang ZHANG

Frontiers in Energy 2022, Volume 16, Issue 5,   Pages 812-821 doi: 10.1007/s11708-020-0669-0

Abstract: The development of highly active nitrogen-doped carbon-based transition metal (M-N-C) compounds for theAmong different M-N-C electrocatalysts, the series of Fe-N-C materials are highly favored because ofFe addition in the second heat treatment usually performed after acid leaching in the catalyst synthesiswill, in turn, guide the design of Fe-N-C materials with enhanced performance.Herein, a series of Fe-N-C electrocatalysts are synthesize and the influence of Fe on the ORR activity

Keywords： oxygen reduction reaction     Fe-N-C     active sites     Fe addition     second heat treatment    

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The performance of nitrate-reducing Fe(II) oxidation processes under variable initial Fe/N ratios: The

Frontiers of Environmental Science & Engineering 2021, Volume 15, Issue 4, doi: 10.1007/s11783-020-1366-2

Abstract:

•Bacterially-mediated coupled N and Fe processes examined in incubation

Keywords： Denitrification     N2O emission     Fe(II) oxidation     Fe/N ratio     Fe minerals    

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Controllable Fe/HCS catalysts in the Fischer-Tropsch synthesis: Effects of crystallization time

Yifei Wang, Shouying Huang, Xinsheng Teng, Hongyu Wang, Jian Wang, Qiao Zhao, Yue Wang, Xinbin Ma

Frontiers of Chemical Science and Engineering 2020, Volume 14, Issue 5,   Pages 802-812 doi: 10.1007/s11705-019-1866-4

Abstract: Among iron carbides, Fe C, as an active phase, has barely been studied due to its thermodynamic instabilityHere, we fabricated a series of Fe C embedded in hollow carbon sphere (HCS) catalysts.species, transmission electron microscopy, X-ray diffraction, N physical adsorption, X-ray photoelectronactivity in the FTS due to its high porosity, appropriate electronic environment, and relatively high FeC content.

Keywords： Fischer–Tropsch synthesis     Fe-based catalyst     Fe2C     hollow carbon sphere     crystallization time    

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Floret-like Fe–N nanoparticle-embedded porous carbon superstructures from a Fe-covalent triazine polymer

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 5,   Pages 525-535 doi: 10.1007/s11705-022-2232-5

Abstract: Fe–Nx nanoparticles-embedded porous carbons with a desirable superstructure have attractedHerein, we employed Fe-coordinated covalent triazine polymer for the fabrication of Fe–Nxto the generation of Fe/N coordination and subsequent Fe–Nx nanoparticles.Owing to the utilization of NaCl crystals, the resultant Fe/N@CNF-800 which was generated by pyrolysisAs expect, the Fe/N@CNF-800 exhibited unexpected oxygen reduction reaction catalytic performance with

Keywords： Fe–Nx nanoparticles     hypersaline-confinement conversion     floret-like carbon     covalent    

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Pd/Fe3O4 supported on bio-waste derived cellulosic-carbon as a nanocatalyst for C–C coupling and electrocatalytic

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 10,   Pages 1514-1525 doi: 10.1007/s11705-022-2158-y

Abstract: 3O4@C) using a simple multi-step process under aerobic conditions.Under mild reaction conditions, the Pd/Fe3O4@C magnetic nanocatalyst demonstratedAlso, the Pd/Fe3O4@C magnetic nanocatalyst exhibited excellent catalytic activityAlso, we explored the use of Pd/Fe3O4@C magnetic nanocatalyst as an electrocatalystInterestingly, the Pd/Fe3O4@C magnetic nanocatalyst exhibited better electrochemical

Keywords： bio-waste     cellulosic-carbon     Pd/Fe3O4     Hiyama cross-coupling     hydrogen evolution    

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Enhancing the efficiency of nitrogen removing bacterial population to a wide range of C:N ratio (1.5:1 to 14:1) for simultaneous C & N removal

Frontiers of Environmental Science & Engineering 2022, Volume 16, Issue 8, doi: 10.1007/s11783-022-1522-y

Abstract:

• Simultaneous C & N removal in Methammox occurs at wide C:N ratio.

Keywords： Methanogens     Biological Nitrogen Removal (BNR)     Simultaneous     Methammox     C:N ratio    

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Probing the catalytic activity of M-N

Fan Ge, Qingan Qiao, Xin Chen, You Wu

Frontiers of Chemical Science and Engineering 2021, Volume 15, Issue 5,   Pages 1206-1216 doi: 10.1007/s11705-020-2017-7

Abstract: In this work, the detailed oxygen reduction reaction (ORR) catalytic performance of M-N O (M= Fe, CoO and Ni-N O , which possess very small overpotentials of 0.27 and 0.32 V, respectively.Such activities are higher than the precious Pt catalyst.Electronic structure analysis reveals one of the reasons for the higher activity of Co-N O and Ni-Nthe density of states reveal that the O doping can improve the electronic structure of the original catalyst

Keywords： M-N-C catalyst     oxygen doping     oxygen reduction reaction     catalytic activity     density functional theory    

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Fe-Mn-sepiolite as an effective heterogeneous Fenton-like catalyst for the decolorization of reactive

Chengyuan SU,Weiguang LI,Xingzhe LIU,Xiaofei HUANG,Xiaodan YU

Frontiers of Environmental Science & Engineering 2016, Volume 10, Issue 1,   Pages 37-45 doi: 10.1007/s11783-014-0729-y

Abstract: A study of the decolorization of reactive brilliant blue in an aqueous solution using Fe-Mn-sepioliteThe Fourier transform infrared (FTIR) spectra of the catalyst showed bending vibrations of the Fe-O.The X-ray diffraction (XRD) patterns of the catalyst showed characteristic diffraction peaks of α-FeO , γ-Fe O and MnO.Moreover, the Fe-Mn-sepiolite catalyst had good stability for the degradation of reactive brilliant blue

Keywords： Fe-Mn-sepiolite catalyst     heterogeneous Fenton-like     reactive brilliant blue     homogeneous precipitation    

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Controllable synthesis of a large TS-1 catalyst for clean epoxidation of a C=C double bond under mild

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 6,   Pages 772-783 doi: 10.1007/s11705-022-2280-x

Abstract: Development of a titanium silicalite-1 (TS-1) catalyst with good crystallinity and a four-coordinateC double bonds.Furthermore, the TS-1#0.1ACh catalyst demonstrated maximum catalytic activity, good selectivity and highImportantly, the TS-1#0.1ACh catalyst was also highly versatile and effective with different unsaturatedC double bonds.

Keywords： size-controlled TS-1     crystal modifier     steam-assisted crystallization     epoxidation    

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Monte Carlo simulation of the PEMFC catalyst layer

WANG Hongxing, CAO Pengzhen, WANG Yuxin

Frontiers of Chemical Science and Engineering 2007, Volume 1, Issue 2,   Pages 146-150 doi: 10.1007/s11705-007-0027-3

Abstract: of the polymer electrolyte membrane fuel cell (PEMFC) is greatly controlled by the structure of the catalystLow catalyst utilization is still a significant obstacle to the commercialization of the PEMFC.on the catalyst utilization and the performance of the PEMFC.The model can predict the effects of some catalyst layer components, such as Pt/C catalyst, electrolyteand gas pores, on the utilization of the catalyst and the cell performance.

Keywords： catalyst utilization     PEMFC     commercialization     Pt/C catalyst     conduction    

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Mass Transfer-Promoted Fe2+/Fe3+ Circulation Steered by 3D Flow-Through Co-Catalyst System Toward Sustainable

Weiyang Lv,Hao Li,Jinhui Wang,Lixin Wang,Zenglong Wu,Yuge Wang,Wenkai Song,Wenkai Cheng,Yuyuan Yao,

Engineering doi: 10.1016/j.eng.2023.06.010

Abstract: from the poor mass/electron transfer and non-durable promotion effect, giving rise to the sluggish Fe2+/Fe3+ cycle and low dynamic concentration of Fe2+ for ROS productionHerein, we present a three-dimensional (3D) macroscale co-catalyst functionalized with MoS2 to achieve ultra-efficient Fe2+ regeneration (equilibrium Fe2+ ratio of 82.4%Our findings highlight an innovative co-catalyst system design to expand the applicability of AOPs based

Keywords： Advanced oxidation processes     3D co-catalyst     Flow-through mode     Enhanced mass transfer     Complex wastewater    

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Effect of noble metal nanoparticle size on C–N bond cleavage performance in hydrodenitrogenation: a study

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 12,   Pages 1986-2000 doi: 10.1007/s11705-023-2337-5

Abstract: Breakage of the C–N bond is a structure sensitive process, and the catalyst size significantly affectsOn the active metal nanoparticle scale, the role of catalyst size in C–N bond cleavage has not been clearlyactivity was evaluated using 1,2,3,4-tetrahydroquinoline and o-propylaniline with different C–N2-hybridized C–N bond cleavage, while the reaction rate tended to increase first and thenC–N bond cleavage.

Keywords： sp3/sp2-hybridized C–N bond     noble metal nanoparticle     catalytic active site     turnover    

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Atomistic simulations of plasma catalytic processes

Erik C. Neyts

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 1,   Pages 145-154 doi: 10.1007/s11705-017-1674-7

Abstract: There is currently a growing interest in the realisation and optimization of hybrid plasma/catalyst systems

Keywords： atomic scale simulation     plasma-catalyst    

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NO hydrogenation to NH over FeCu/TiO catalyst with improved activity

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 12,   Pages 1973-1985 doi: 10.1007/s11705-023-2364-2

Abstract: Hence, developing an efficient and environmentally friendly catalyst is imperative.Notably, the optimized 10Fe-8Cu/TiO2 catalyst exhibited exceptional catalytic performancerate exceeding 80% and an NH3 selectivity exceeding 98% at atmospheric pressure and 350 °C.

Keywords： NO hydrogenation     synthetic ammonia     10Fe-xCu/TiO2     high selectivity    

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Title Author Date Type Operation

New insight into effect of potential on degradation of Fe-N-C catalyst for ORR

Yanyan GAO, Manman QI, Liang HE, Haiping CHEN, Wenzhe LUO, Ming HOU, Zhigang SHAO

Journal Article

Influence of Fe on electrocatalytic activity of iron-nitrogen-doped carbon materials toward oxygen reduction

Lin LI, Cehuang FU, Shuiyun SHEN, Fangling JIANG, Guanghua WEI, Junliang ZHANG

Journal Article

The performance of nitrate-reducing Fe(II) oxidation processes under variable initial Fe/N ratios: The

Journal Article

Controllable Fe/HCS catalysts in the Fischer-Tropsch synthesis: Effects of crystallization time

Yifei Wang, Shouying Huang, Xinsheng Teng, Hongyu Wang, Jian Wang, Qiao Zhao, Yue Wang, Xinbin Ma

Journal Article

Floret-like Fe–N nanoparticle-embedded porous carbon superstructures from a Fe-covalent triazine polymer

Journal Article

Pd/Fe3O4 supported on bio-waste derived cellulosic-carbon as a nanocatalyst for C–C coupling and electrocatalytic

Journal Article

Enhancing the efficiency of nitrogen removing bacterial population to a wide range of C:N ratio (1.5:1 to 14:1) for simultaneous C & N removal

Journal Article

Probing the catalytic activity of M-N

Fan Ge, Qingan Qiao, Xin Chen, You Wu

Journal Article

Fe-Mn-sepiolite as an effective heterogeneous Fenton-like catalyst for the decolorization of reactive

Chengyuan SU,Weiguang LI,Xingzhe LIU,Xiaofei HUANG,Xiaodan YU

Journal Article

Controllable synthesis of a large TS-1 catalyst for clean epoxidation of a C=C double bond under mild

Journal Article

Monte Carlo simulation of the PEMFC catalyst layer

WANG Hongxing, CAO Pengzhen, WANG Yuxin

Journal Article

Mass Transfer-Promoted Fe2+/Fe3+ Circulation Steered by 3D Flow-Through Co-Catalyst System Toward Sustainable

Weiyang Lv,Hao Li,Jinhui Wang,Lixin Wang,Zenglong Wu,Yuge Wang,Wenkai Song,Wenkai Cheng,Yuyuan Yao,

Journal Article

Effect of noble metal nanoparticle size on C–N bond cleavage performance in hydrodenitrogenation: a study

Journal Article

Atomistic simulations of plasma catalytic processes

Erik C. Neyts

Journal Article

NO hydrogenation to NH over FeCu/TiO catalyst with improved activity

Journal Article